Hall Angle

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https://doi.org/10.1038/s41467-021-22857-y OPEN

Deriving the skyrmion Hall angle from skyrmion


lattice dynamics
R. Brearton 1,2 ✉, L. A. Turnbull 3, J. A. T. Verezhak4, G. Balakrishnan 4, P. D. Hatton 3,

G. van der Laan 2 ✉ & T. Hesjedal 1 ✉


1234567890():,;

Magnetic skyrmions are topologically non-trivial, swirling magnetization textures that form
lattices in helimagnetic materials. These magnetic nanoparticles show promise as high effi-
ciency next-generation information carriers, with dynamics that are governed by their
topology. Among the many unusual properties of skyrmions is the tendency of their direction
of motion to deviate from that of a driving force; the angle by which they diverge is a
materials constant, known as the skyrmion Hall angle. In magnetic multilayer systems, where
skyrmions often appear individually, not arranging themselves in a lattice, this deflection
angle can be easily measured by tracing the real space motion of individual skyrmions. Here
we describe a reciprocal space technique which can be used to determine the skyrmion Hall
angle in the skyrmion lattice state, leveraging the properties of the skyrmion lattice under a
shear drive. We demonstrate this procedure to yield a quantitative measurement of the
skyrmion Hall angle in the room-temperature skyrmion system FeGe, shearing the skyrmion
lattice with the magnetic field gradient generated by a single turn Oersted wire.

1 Department of Physics, Clarendon Laboratory, University of Oxford, Oxford, UK. 2 Diamond Light Source, Harwell Science and Innovation Campus, Didcot, UK.
3 Department of Physics, Durham University, Durham, UK. 4 Department of Physics, University of Warwick, Coventry, UK. ✉email: [email protected];

[email protected]; [email protected]

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M
agnetic skyrmions (skyrmions hereafter) are topologi- shown to be much less strongly affected by pinning potentials; in
cally robust, localized whirls of magnetization1–4—a this case, the skyrmion Hall angle typically approaches 90°5.
simulated image of an isolated magnetic skyrmion is Furthermore, skyrmions with these properties are expected to
shown in Fig. 1a. The topology of a skyrmion gives rise to a enjoy significantly reduced depinning thresholds10,11, and can be
Magnus term in its equation of motion5. As a result, skyrmions used in device architectures that are incompatible with typical
are generally driven at an angle to the direction of applied forces; force–velocity relationships12.
the relationship between driving force, induced velocity and the While in many respects a skyrmion Hall angle near to 90° is
skyrmion Hall angle is indicated in Fig. 1b. The stability and beneficial, this is not always the case. In device schematics which
mobility of skyrmions have inspired the design and manufacture require skyrmions to be driven along a straight line, it would be
of a multitude of skyrmion-based devices; despite this, the desirable for skyrmions to not veer from their path. Non-zero
widespread adoption of magnetic skyrmions in computational skyrmion Hall angles deflect skyrmions towards the boundary of
schemes is far from reality6–9. For the purposes of device man- the structure where they can be trapped or destroyed13. This led
ufacturing, the magnitude of the skyrmion Hall angle must be to a surge of recent interest in skyrmions in antiferromagnetic,
accurately obtained on a material-by-material basis. This is synthetic antiferromagnetic and compensated ferrimagnetic
necessary as the skyrmion Hall angle completely dictates the materials, which have a skyrmion Hall angle of 0°14–16.
qualitative dynamical properties of skyrmions in a system, and as This difference in qualitative behaviour makes the quantitative
variations in, e.g., material quality, doping and surface treatment, determination of the skyrmion Hall angle an important topic; one
can alter the many parameters that control the magnitude of the which has been well tackled for the case of skyrmions in magnetic
skyrmion Hall angle (such as density of pinning sites, damping heterostructures16–21. In these systems, skyrmions tend to be
and anisotropies) in a manner that is difficult to predict. sparse, and their controlled nucleation has been well studied22.
For instance, skyrmions for which the Magnus force is large This makes the isolation and manipulation of individual sky-
compared to other terms in their equation of motion have been rmions possible, allowing the skyrmion Hall angle to be obtained
by tracing the real space motion of skyrmions under the influence
of a driving force21. Such techniques are inapplicable to the study
of the skyrmion lattice state, where individual skyrmions cannot
readily be labelled or tracked in real space, or where skyrmions
are too small to be resolved with the required time resolution.
Here, we report a study of the signatures of lattice dynamics in
reciprocal space, showing that the motion of dislocations through
a sheared skyrmion lattice forces the lattice to reorient along its
direction of motion. The shear applied to the skyrmion lattice
also leads to a build-up of strain, which when combined with the
lattice reorientation, allows for the unambiguous measurement of
the skyrmion Hall angle in reciprocal space.

Results
The high-temperature skyrmion system FeGe. A particularly
interesting chiral magnet is the widely studied FeGe, an itinerant
helimagnet which hosts sub-100 nm diameter skyrmions near
room-temperature23. Despite the wealth of research carried out
on this material, measurements of the skyrmion Hall angle in
FeGe have remained elusive. To experimentally measure the
skyrmion Hall angle in FeGe, we set up a shear force with the
stray magnetic field from a current-carrying wire, studying the
reciprocal space dynamics using resonant elastic X-ray scattering
(REXS)24.

The effect of shear stress on two-dimensional crystals. To


determine the skyrmion Hall angle from reciprocal space mea-
surements, it is necessary to understand the signature of real
space motion in the structure factor. For homogeneous drives,
this has been studied in detail, though none of the rich dynamic
phases explored in the literature allow for the unambiguous
determination of the skyrmion Hall angle from the structure
factor alone10,25. To move beyond this limitation, it is lucrative to
borrow results from the study of crystals under strain. In this
case, the properties of a crystal are dictated entirely by its defects
Fig. 1 Magnetic skyrmions. a Magnetisation distribution of an isolated and dislocations26—an excellent classical example of this is the
magnetic skyrmion. The magnetic moments far from the centre point shear stress required to plastically deform a crystal. In 1926, it was
antiparallel to the central spin, with intermediate moments winding away calculated by Frenkel that the shear stress required for plastic
from the centre in case of a Bloch-type skyrmion (and point radially in case deformation of a lattice should be on the order of its shear
of a Neel-type skyrmion). b When a skyrmion is driven by an applied force modulus27. In reality, experimental values are 4–8 orders of
F, it moves with a velocity v at an angle θSkH to the direction of the applied magnitude smaller28. The reason for this stark discrepancy is the
force. This angle is constrained to lie in the closed interval ½90 ; 90 , i.e., existence of dislocations in a real lattice. The shear stress required
skyrmions cannot be driven backwards by a force that acts forwards. to plastically deform a real lattice is instead on the order of the

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Peierls–Nabarro stress, i.e., the shear stress required to displace a Shearing a skyrmion lattice with a magnetic field gradient. To
dislocation29. apply a shear stress to a skyrmion lattice, the sample was
As an ideal skyrmion lattice state is two-dimensional (extend- immersed in a non-uniform magnetic field. Assuming that the
ing as tubes in depth30,31), the only form of dislocation present in magnetic field varies slowly over the length scale of a single
~
 the Zeeman energy of a skyrmion at position R ¼
the lattice are edge dislocations, which typically manifest skyrmion,
themselves in hexagonal 2D materials as 5–7 defects32. These 
x; y; z can be written as
5–7 defects can glide in the direction of their Burgers vector for
very little energy28. The allowed Burgers vectors for 5–7 defects EZeeman ð~
RÞ ¼ ~ Bð~
RÞ  I Sk ; ð1Þ
are real primitive lattice vectors, confining defect glides to three R
special axes. If a shear stress is applied whose direction is not where we defined I Sk ¼ A m r ~
~ Sk ð~ RÞdA. Here, m ~ Sk is the
Sk
parallel to one of the three axes, motion is possible only by magnetization configuration of a skyrmion and the integral is
combining glides and climbs. An example visualization of such a taken over the area ASk bounded by the skyrmion’s radius. In the
defect in a skyrmion lattice, including its Burgers vector, is shown measurements, a constant magnetic field ~ B0 ¼ B0 ^z was applied by
in Fig. 2a. permanent magnets, on top of which a perturbative non-uniform
The climbing motion of 5–7 defects is much more costly than magnetic field was generated from a single turn of wire. This gives
glides, as each climb changes the macroscopic shape of the rise to a field profile which can be written as
crystal28. If the direction of a shear force is at an angle θ from one
of the glide axes, in order to plastically deform the crystal, there Bz ðyÞ ¼ B0 þ B1 =y; ð2Þ
must be sin θ defect climbs for every cos θ defect glides. As such, where the wire lies along the x-axis in the Cartesian coordinate
the system must spend an energy EClimb sin θ þ EGlide cos θ to system (cf. Oersted wire in Fig. 3). This leads to a force Fy =
propagate a defect when relieving strain, where EClimb ≫ EGlide. ISkB1/y2 acting on the skyrmion lattice.
This creates an effective energy cost EDefect ¼ K sin θ when a 2D The steady-state motion of a skyrmion under the influence of a
crystal is misoriented by an angle θ to the direction of an applied driving force is well described by the Thiele equation, given by35
shear, where K is a constant of proportionality that is
proportional to the energy cost of an individual defect climb ~ v ¼~
F M  α~ F ext ¼ I Sk B1 ^y=y2 ; ð3Þ
(which is proportional to the number of particles in the crystal)
where α is the damping coefficient, ~ v is the velocity of the
and the magnitude of the applied shear. To minimize this
energy contribution, it is overwhelmingly preferential for a 2D skyrmion, and ~F ext is the external force that acts on the skyrmion.
crystal to rotate until it is aligned along the direction of an The Magnus force ~ F M can be written as ~ FM ¼ ~ G ´~v and it acts
applied shear. In real space, this would correspond to a shear perpendicularly to the direction of the applied velocity, where
force acting vertically in Fig. 2a, in which case strain can be easily ~
G ¼ ± 2πN^z is the gyrovector. Here, the topological winding
relieved by propagation of the pictured dislocation along its number N is the number of times the skyrmion moments wrap
Burgers vector. the unit sphere. The angle from the y-axis at which skyrmions are
As such, 2D crystals make two key responses to shear forces driven is given by
which are observable in their scattering structure factor. Firstly,
θSkH ¼ arctanðG=αÞ: ð4Þ
the crystal responds by reorienting itself so that the crystal’s real
lattice vectors are collinear with the shear direction. Secondly, the Figure 3 shows velocity fields obtained from solutions of Eq.
shear introduces a uniaxial distortion of the structure factor peaks (3) as a function of θSkH. These velocity fields shear the skyrmion
which indicates the direction of motion; this distortion is visible lattice along its direction of motion. The direction of the shear
in Fig. 2b. Such distortions are known to occur in sheared can be inferred from the structure factor, and the direction of the
colloidal suspensions, and have been recently studied in skyrmion force is known; the skyrmion Hall angle is then the angle between
systems33,34. the shear and the applied force.

Fig. 2 Skyrmion lattice defects. a Visualisation of an edge dislocation in a skyrmion crystal. This dislocation manifests itself as a topological defect, which
can be thought of as one skyrmion gaining a nearest neighbour from an adjacent skyrmion; the Voronoi cells surrounding the skyrmions with 5 and 7
nearest neighbours are coloured yellow and green, respectively. This so-called 5–7 defect can glide along its Burgers vector, indicated by b, costing very
little energy. The Burgers vector of a 5–7 defect must lie along a real lattice basis vector28. Were the lattice sheared vertically, strain could be efficiently
relieved by propagation of the pictured 5–7 defect along its Burgers vector. b Idealized visualization of the diffraction pattern from a strained 2D crystal with
a 5–7 defect. Strain in the vicinity of the defect elongates four of the peaks anisotropically: the Burgers vector specifies a unique direction and its
corresponding defect breaks the six-fold symmetry of the hexagonal lattice34.

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Fig. 3 Sheared skyrmion lattices in a perturbative linear field gradient for materials with different skyrmion Hall angles. a The red arrows indicate the
magnitude and direction of the induced velocity as a function of distance from the current-carrying Oersted wire and the skyrmion Hall angle θ. b For all
finite skyrmion Hall angles, the velocity field induced by the field gradient shears the skyrmion lattice along its direction of motion. This shear leads to
lattice reorientation and uniaxial peak broadening, indicated in the magnetic structure factors provided beneath their corresponding shear field cartoons. As
the direction of the applied force is known, and the direction of the induced motion can be inferred from the structure factor, the skyrmion Hall angle can be
acquired by measuring the angle between these two vectors.

REXS measurements of the skyrmion Hall angle. To use this damping. The skyrmion Hall angle in such candidate low-
approach to measure the skyrmion Hall angle experimentally, REXS dissipation materials can be measured using the presented tech-
was performed in transmission on a thin, 10 × 10-μm2-sized FeGe nique, unlocking the possibility of developing ultra-high mobility
lamella with a measured TC of 273 K31. The presence of stray devices which take advantage of this unique motion10–12.
temperature or magnetic field gradients is known to cause the Recent theoretical work suggests that the presence of pinning
skyrmion lattice to rotate12,36. To verify that no such unintended potentials in real materials should make the skyrmion Hall angle
external forces were present in our experimental setup, the motion dependent on the magnitude of an applied drive, approaching
of the peaks in the REXS diffraction pattern was tracked prior to the zero in the low drive limit, while the value given in Eq. (4) is
application of the shearing magnetic field gradient. This motion was expected to correspond to the high drive limit10,11. This
found to be very small, and can be seen by comparing Fig. 4a and b. hypothesis is supported by experimental evidence, obtained by
Subsequently, the response of the skyrmion lattice to the application measuring the skyrmion Hall angle in sputtered magnetic
of a shearing magnetic field gradient was measured; the average of multilayers17. The highly energetic nature of the sputtering
the diffraction patterns obtained after this drive is shown in Fig. 4c. technique is expected to be the source of the pinning potentials
An example video of the response of the skyrmion lattice to the present in these materials systems17. As the FeGe lamella used in
shearing magnetic field is included in the Supplementary Material this experiment was cut from a high-quality single crystal31, we
(Supplementary Video 1), as well as a video of the average response anticipate that this drive dependence will be suppressed in our
(Supplementary Video 2). sample, and that the angle measured here should be considered to
While these data make the reorientation of the skyrmion lattice be a lower bound that is close to the theoretical value. A detailed
in response to a shear force strikingly clear, the six-fold symmetry study of the drive dependence of the skyrmion Hall angle in
of the acquired diffraction pattern made the unambiguous samples cut from a single crystal would make for an interesting
determination of the skyrmion Hall angle impossible. To break topic of future research.
this symmetry, sufficient strain must build up in the skyrmion This technique also opens up the prospect of studying the effect
lattice in response to the shear to broaden the diffraction peaks34. of chemical doping on the skyrmion Hall angle in a precise and
Leveraging the reduction in magnetic softness further from TC, systematic manner. The ability to fine tune the response of a
the same experiment was performed at 250 K; the results are skyrmion to an applied force represents a significant milestone in
shown in Fig. 4d. The angle between the labelled direction of the field of skyrmionics, moving the skyrmion Hall angle from an
motion and the direction of the applied force is the skyrmion Hall unknown variable to a free parameter. The direction of motion of
angle, and was measured to be 55° ± 2°. skyrmions can be further controlled by exploiting the direction in
which external forces are applied. While the skyrmion Hall angle
is defined as the angle between an applied force and a skyrmion’s
Discussion resultant velocity, the direction in which forces are applied can be
This angle is larger than any previous measurement of the sky- complicated by the internal structure of skyrmions. In Eq. (3), the
rmion Hall angle in magnetic multilayer systems. However, this is external force ~
F ext is set to be equal to the gradient of the Zeeman
still far from the theoretical limit of 90°. The primary damping energy of a skyrmion. When ~ F ext is instead equated to the force
mechanism for skyrmions moving through a metal occurs via due to spin-orbit torque from an adjacent heavy metal layer, the
interaction with conduction electrons37. An insulating skyrmion- Thiele equation becomes
hosting material (such as Cu2OSeO3) may have a skyrmion Hall
~ v ¼ kRðϕÞ~jHM
F M  α~ ð5Þ
angle which is closer to the 90° limit, due to greatly reduced

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Fig. 4 Experimental determination of the skyrmion Hall angle of FeGe. First, the temperature was set to 268 K (TC =273 K) and a skyrmion-stabilising
magnetic field was applied to reach the skyrmion phase pocket. The resonant elastic X-ray scattering (REXS) pattern in a shows the typical signature of a
skyrmion lattice containing several domains, with multiple sets of six-fold symmetric peaks, see ‘Methods’ for details. b In order to assure stable starting
conditions without uncontrolled lattice reorientation, the diffraction experiment was repeated after a sufficient waiting period (15 min), showing a virtually
identical pattern. c After applying a linear field gradient (I on) for 15 min, the shear force (F) introduced by the field gradient drives the skyrmion lattice to
completely reorient along its direction of motion, resulting in single, six-fold symmetric spot pattern. A video of the evolution from a to b to c is provided in
the Supplementary Materials (Supplementary Video 1). Owing to its six-fold symmetry, there are three possible directions of motion that result in the same
diffraction pattern: v1 at 55°, v2 at −5°, and v3 at −65° (note that the skyrmion Hall angle is restricted to [−90°, 90°]). In order to resolve this ambiguity,
the stiffness of the skyrmion lattice was tuned from its soft state just below TC to a harder lattice at a reduced temperature of 250 K, in which strain can
build up. d The final orientation of the skyrmion lattice is generally the same as for the soft lattice shown in (c), however, now the presence of strain leads
to a characteristic anisotropic peak broadening (highlighted and magnified, see red ellipse; note that another pair of broadened peaks is masked by the
beamstop). The direction of peak broadening is consistent with v1 and a Hall angle of 55°, as shown in the simulated REXS pattern in the inset in the top
right for which the direction of the shear is 55∘ away from the direction of the applied force.

where k is a constant of proportionality, R(ϕ) is the rotation Magnetic gradient field. To provide the perturbative field, a single turn of 600-
matrix in the plane spanned by ~F M and ~
v, ϕ is the helicity angle of μm-diameter Kapton-insulated Cu wire was suspended ~1 mm from the sample,
a skyrmion and ~jHM is the current density in the heavy metal
with the core of the wire approximately lying in the plane of the sample surface. An
out-of-plane magnetic field gradient of ~1 mT mm−1 was mapped out with a Hall
layer7. As Bloch-type skyrmions have a helicity of ±π/2, the force probe, obtained by driving 11 A through the wire. The wire was thermally
due to spin-orbit torque is normal to ~jHM ; in this case, the anchored on points, each ~ 10 mm away on both from the sample, and the
direction of the skyrmion’s induced velocity is parallel to~jHM only experiment was performed under ultrahigh vacuum conditions, which minimizes
the effects of a perturbative temperature gradient.
when the skyrmion Hall angle is 90°. A detailed discussion of the Entering the skyrmion phase by field sweeping from the helical state, a roughly
relationship between current, force and drive direction for Néel- randomly oriented skyrmion lattice was obtained. Due to the nature of the small
and Bloch-type skyrmions can be found in ref. 7. 10 × 10 μm2 FeGe samples (prepared by focused-ion-beam milling) there were
In conclusion, we have introduced a novel technique for the preferential orientations for the skyrmion lattice in the absence of a driving force,
which could be the result of, e.g., a strong shape anisotropy. As a result of this
straightforward measurement of the skyrmion Hall angle in energetic anisotropy, we observed minor natural reorientation of the skyrmion
skyrmion lattice systems. The success of the technique demon- lattice for 1–2 min upon entering the skyrmion pocket in the absence of any
strates that even the properties of a crystal consisting of topolo- external drive. In order to completely rule out any effects due to this reorientation,
gically wound magnetic moments are completely determined by we found that waiting for 15 min was sufficient. The field gradient was applied
after this 15 min pause and the lattice reorientation was measured for a further
its defects and dislocations, mirroring the discovery of the 15 min. This experiment was performed 15 times at 268 K on a sample of FeGe
Peierls–Nabarro stress. We have used this technique to measure with a measured TC of 273 K: four times with an out-of-plane magnetic field
the skyrmion Hall angle in a thin lamella of FeGe, finding an of 55 mT, four times at 50 mT, four times at 45 mT, and three times at 60 mT.
angle of 55° ± 2°. This angle far exceeds previous measurements The reorientation in response to the application of the shearing Oersted field
was found to be independent of the out-of-plane magnetic field and was
of the skyrmion Hall angle in magnetic multilayer systems, pro- extremely significant in all experiments. The average overall 15 final states is
viding verification for previous theoretical work38. This giant shown in Fig. 4c.
skyrmion Hall angle opens the door to ultra-low dissipation The same experiment was then repeated 24 times at 250 K, eight times each at
devices, while the technique allows for the methodical study of external magnetic field value of 65, 60, and 55 mT. An average over the final frames
the skyrmion Hall angle in the skyrmion lattice state. obtained after application of the magnetic field gradient for 15 min at 250 K is
given in Fig. 4d, with the anisotropic peak broadening indicating the rough
direction of motion.
The skyrmion Hall angle was calculated from the data set acquired just below TC
Methods at 268 K, as shown in Fig. 4c. Measuring at this temperature has the advantage that
Resonant elastic X-ray scattering. The REXS experiment was carried out in the the same information can be obtained in a shorter period of time, as compared to
transmission geometry on a 400-nm-thick, 10 × 10 μm2-sized FeGe lamella using a measuring at a lower temperature. As such, the strain induced anisotropy measured in
CCD camera31. To protect the camera from overexposure in this geometry, a the 250 K experiment was used to infer the approximate direction of motion,
horizontal beamstop was used to block the direct X-ray beam. Nevertheless, the while the precise measurement of the skyrmion Hall angle was made using the
Airy rings which arise from optical diffraction of the beam are extremely bright. diffraction spots imaged in Fig. 4c. The quoted uncertainty in the measured value
These, alongside other contributions from the direct beam, have been masked in all is half of the angular width of the average overall 15 final peak orientations imaged
figures to emphasize the magnetic diffraction signal. in Fig. 4c.

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