Z.G. Wang, H.T. Bi and C.J. Lim Fluidization Research Centre Department of Chemical and Biological Engineering University of British Columbia Vancouver, BC, V6T 1Z4, Canada
Z.G. Wang, H.T. Bi and C.J. Lim Fluidization Research Centre Department of Chemical and Biological Engineering University of British Columbia Vancouver, BC, V6T 1Z4, Canada
Z.G. Wang, H.T. Bi and C.J. Lim Fluidization Research Centre Department of Chemical and Biological Engineering University of British Columbia Vancouver, BC, V6T 1Z4, Canada
v
t
q
q q
(1)
where
vq
is the velocity of phase q;
q
is the volume fraction of phase q, and the following
condition holds.
1
1
=
=
n
q
q
(2)
where n is the total number of phases, and n=2 in our simulation.
Conservation equation of momentum:
For the fluid phase l:
) ( ) ( ) (
v v
K
g P
v v v
t
l s
sl
l
l
l
l
l l l
l
l l
l
+ + + = +
(3)
For the solid phase s:
S v v
K
g
P
P
v v v
t
s s l
ls
s
s
s
s s
s s s
s
s s
s
+ + + + = +
) ( ) ( ) (
(4)
where
l
is the density of the fluid phase, P is the static pressure shared by all phases,
l
is
the fluid phase stress-strain tensor, g is the gravitational acceleration, K
ls
=K
sl
is the
momentum exchange coefficient between fluid phase l and solid phase s,
s
is the density of
the particle,
s
is the solid phase stress-strain tensor, P
s
is the solid pressure,
Ss
is the solid
phase source term.
The stress-strain tensor for phase q:
I
v v v
q q
q q
T
q q q
q
q
+ + = )
3
2
( ) (
(5)
where
q
and
q
are the shear and bulk viscosity of phase q.
For the solid phase s, the solids shear viscosity is the sum of the collisional viscosity,
kinetic viscosity and the optional frictional viscosity, as shown in equation (6).
+
+ =
fr s kin s col s s , , ,
(6)
The collision viscosity is modeled as:
) (
) 1 (
5
4
2 1
, 0 ,
+ =
s
ss
ss
s
s
s
col s
e
g
d
(7)
where d
s
is the diameter of the solid particles, g
0,ss
is the radial distribution function, and
FLUENT employs the following expression as equation (8), e
ss
is the coefficient of restitution,
s
is the granular temperature.
(
(
=
|
|
|
.
|
\
|
max ,
3 1
1
, 0
1
s
s
ss
g
(8)
The following expression from Gidaspow (1994) is used to estimate the kinetic
viscosity.
(
+ +
+
= ) 1 (
5
4
1
) 1 ( 96
10
, 0
2
, 0
,
e
g
g
e
d
ss s
ss
ss
ss s
s s s
kin s
(9)
In our simulation, the frictional viscosity was not considered, and the solid bulk
viscosity used either the following form from Lun et al. (1984) or a constant value of zero.
) (
) 1 (
3
4
2 1
, 0
+ =
s
ss
ss
s
s
s s e
g
d
(10)
Fluid-solid exchange coefficients:
The fluid-solid exchange coefficient K
sl
can be written in the following general form:
s
s
s
sl
f
K
=
(11)
where f is defined differently for the different exchange coefficient models, and
s
, the
particulate relaxation time, is defined as
18
2
l
s s
s
d
=
(12)
In FLUENT, there are three models for fluid-solid exchange coefficient, and the
Gidaspow drag model is applied in this work.
Gidaspow drag model (1994):
The Gidaspow model is a combination of the Wen and Yu model (1966) and the Ergun
(1952) equation.
When
8 . 0 >
l
, the fluid-solid exchange coefficient K
sl
is of the following form:
65 . 2
4
3
=
l
s
l s
l
l
s
D sl
d
v v
C K
(13)
where,
(
+ = )
Re
( 15 . 0 1
Re
24
687 . 0
s
l
s
l
D
C
(14)
l
l s s l
s
v v d
=
Re
(15)
When
8 . 0
l
d
v v
d
K
s
l s
s
l
s
l
l
l s
sl
75 . 1
) 1 (
150
2
(16)
Solids Pressure:
For granular flows in the compressible regime (i.e., where the solids volume fraction is
less than its maximum allowed value), a solids pressure is calculated independently and used
for the pressure gradient term,
P
s
+ +
=
s
ss
s ss
s
s
s
s s
g
e P
, 0
2
) 1 ( 2
(17)
The solid phase source term:
It was found that the ratio of the pressure drop at stable spouting to the pressure drop
at stable fluidization is usually smaller than one for both the cylindrical spouted beds and the
conical spouted beds (Mathur and Epstein, 1974; Mukhlenov and Groshtein, 1964, 1965). At
partial spouting state, however, the above ratio is usually bigger than one in the ascending
process. Thus, the gravity term in the axial solid phase momentum equation, equation (4),
needs to be modified. To do so, a solid phase source term, S
s,a
, is introduced into the axial
solid phase momentum equation for both the spout and annulus regions:
When
8 . 0
l
and
H
Z
0
) 1 ( ) (
,
= + =
(18)
When
8 . 0 >
l
(in the spout and the fountain)
g
k
g
k
g
S
s
s s
s
s s
s
s a s
) 1 ( ) (
,
= + =
(19)
where Z is the axial height, H
0
is the static bed height, k
a
and k
s
are the ratio of the pressure
drop of spouted beds to the pressure drop at stable fluidization, which are functions of
operating conditions and the geometrical structure of the bed. In the gas velocity ascending
process, when the spouted bed is operated at partial spouting state, k
a
is usually greater than
one. To simplify the problem, k
s
was usually set to one.
By applying the above solid phase source term, it is possible to use FLUENT to
simulate a spouted bed operated at partial spouting or stable spouting state for both the
ascending and the descending processes.
3. Simulating Conditions
Table 1. List of simulation conditions
Description Value Comment
Operating gas velocity, U
i
24 m/s Based on D
i
Gas density,
l
1.225 kg/m
3
Air
Gas viscosity,
l
1.789410
-5
kg/(ms) Air
Particle density,
s
2500 kg/m
3
Spherical glass beads
Particle diameter, d
s
0.00116 m Uniform distribution
Initial solid packing,
s,0
0.61 Fixed value
Packing limit,
s,max
0.61 Fixed value
Solid viscosity,
s
Gidaspow Eq. (7) + Eq. (9)
Solid bulk viscosity (Base case),
s
0 Fixed value
Cone angle, 45 Fixed value
Diameter of the upper section, D
c
0.45 m Fixed value
Total height of the column 1.6 m Fixed value
Gas inlet diameter, D
0
0.019 m Fixed value
Diameter of the bed bottom, D
i
0.038 m Fixed value
Static bed height, H
0
0.396 m Fixed value
Solver
2 dimensional, double precision, segregated,
unsteady, 1
st
order implicit, axisymmetric
Multiphase Model Eulerian Model, 2 phases
Viscous Model Laminar model
Phase Interaction (Base case)
Fluid-solid exchange coefficient: Gidaspow Model
Restitution coefficient: 0.9
Time steps (Final value) 0.00001s Fixed value
Convergence criterion 10
-3
Default in FLUENT
Table 2. Boundary conditions
Description Comment
Three types of radial distributions are tested for fluid phase
Inlet
No particles enter for solid phase
Uniform velocity distribution for fluid phase
Outlet
No particle exits for solid phase
Axis Axisymmetric
Non-slip for fluid phase
Wall
Zero shear stress for solid phase
In the simulation, the bed geometrical structure and dimensions (as shown in Fig. 1
(b)), the spouting gas, the bed material as well as operating conditions used are kept almost
the same as in the actual experiment. The operating gas velocity used in simulations is about
2% higher than the experiment, and the total column height is much longer than the actual
experimental setup. Because of the influence of the outlet structure on flow field, comparisons
between the experiment and simulation will not be considered above the bed surface. Details
on simulation conditions are listed in Table 1, with boundary conditions given in Table 2.
In order to investigate all possible factors that may affect simulation results, parameters
such as the fluid inlet velocity profile, solid bulk viscosity, restitution coefficient, exchange
coefficient and the source term are selected for the sensitivity analysis. At the same time, three
kinds of mesh/grid partitions of the bed are also studied. All conditions investigated are
summarized in Table 3.
Table 3. Summary of conditions used for sensitivity analysis
Grid
Partition
Fluid Inlet
Radial Profile
Bulk
Viscosity
Restitution
Coefficient
Exchange
Coefficient
Source
Term
Uniform
Parabolic
0
Lun et al.
0.9
0.81
0.99
K
sl
(Gidaspow)
0.8* K
sl
(Gidaspow)
1.2* K
sl
(Gidaspow)
k
a
=1.0
k
a
=0.7
k
a
=0.5
k
a
= k
s
=0.5
Partition 1
(10497 cells)
k
a
=0.41
k
a
=1.0
k
a
=0.7
Partition 2
(4102 cells)
k
a
=0.5
k
a
=1.0
k
a
=0.7
Partition 3
(2598 cells)
1/7
th
power law
0
0.9
K
sl
(Gidaspow)
k
a
=0.5
Notes: a. In simulations, k
s
equals to1.0 unless having further indications;
b. Conditions for the base case are as follows: partition 1; parabolic fluid inlet profile; zero value of the
solid bulk viscosity; restitution coefficient equals to 0.9; fluid-solid exchange coefficient estimated by the
Gidaspow model, k
a
equals to1.0.
4. Experiments
Experiment was conducted in two conical spouted to generate data for the validation
of the simulation results. A schematic diagram of the experimental unit is shown in Fig. 1 (a).
Conical spouted beds (both a semi-circular half column and a full column) are made of
Plexiglas with an included angle of 45
o
. The diameter at the conical base D
i
is 0.038 m, the
diameter of the nozzle D
0
is 0.019 m, and the diameter of the upper cylindrical section D
c
is
0.45 m. Glass beads of 0.00116 m in diameter were used as the bed material, compressed air
at the ambient temperature was used as the spouting gas. Other particle properties and
detailed operating conditions are shown in Table 4.
(a) (b)
Fig. 1. Schematic drawing of the Plexiglas conical spouted bed unit.
Table 4. Particle properties and operating conditions
Particle diameter
d
s
, (m)
Particle density
s
, (kg/m
3
)
Lose-packed
voidage,
l,0
Geldarts
classification
Static bed height
H
0
, (m)
Velocity
U
i
, (m/s)
0.00116 2500 0.39 D 0.396 23.5
The distribution of the static pressure was measured by static pressure probes
connected to differential pressure transducers; the distribution of the vertical solid velocity and
solid hold up were measured by optical fiber probes which were calibrated separately in
advance. During experiments, all probes can be radially traversed to measure the profile at
each vertical position.
5. Results and Discussion
Notes for Fig. 2 to Fig. 7:
Figure (a) Figure (b)
Red lines: Z=38mm; Blue lines: Z=89mm;
Magenta lines: Z=191mm; Cyan lines: Z=292mm
Red lines: Z=140mm; Blue lines: Z=241mm
Magenta lines: Z=343mm
The grid partition
The effect of grid size or grid partition on the simulation results is first examined by
comparing the simulation results from three grid sizes. As shown in Figure 2, the grid size
within the range investigated in the current simulation has little effect on the radial distribution
of the static pressure, although some influence on the distribution of the axial solid velocity is
observed, especially in the spout region. Thus, the more accurate grid partition with the
smallest grid size, partition 1, was used in the following sensitivity analysis. It is also seen from
Fig. 2 that simulated results on the axial solid velocity agree very well with experimental data,
but not for the static pressure profile under the base operating conditions without the
consideration of the solid phase source term.
0.00 0.04 0.08 0.12 0.16
r (m)
0
1000
2000
3000
4000
5000
6000
P
(
P
a
)
292
191
89
38
Z(mm)
0.00 0.02 0.04 0.06 0.08
r (m)
-2.0
0.0
2.0
4.0
6.0
8.0
10.0
V
s
(
m
/
s
)
140
241
343
Z(mm)
(a) (b)
Fig. 2. Comparison between experimental results and simulated results with different grid
partitions at k
a
=1.0 (k
s
=1.0, 1/7
th
power law). Symbols are experimental results, and lines are
simulated results. (Solid lines correspond to partition 1, dotted dash lines correspond to
partition 2, dash lines correspond to partition 3.)
The fluid inlet profile
The influence of fluid inlet profiles on the simulation result is shown in Fig. 3. Although
fluid inlet profiles have little effect on the distribution of the static pressure, the influence on the
distribution of the axial solid velocity is shown clearly, especially in the spout region. Simulated
static pressures overestimated experimental data significantly when k
a
was chosen to be equal
to 1.0, although the simulated particle velocity profile is quite close to the experimental data
except for the case when a parabolic inlet gas velocity profile was used. Therefore, 1/7
th
power
law or turbulent distribution inlet velocity profile was used in subsequent simulations.
0.00 0.04 0.08 0.12 0.16
r (m)
0
1000
2000
3000
4000
5000
6000
P
(
P
a
)
292
191
89
38
Z(mm)
0.00 0.02 0.04 0.06 0.08
r (m)
-2.0
0.0
2.0
4.0
6.0
8.0
10.0
12.0
V
s
(
m
/
s
)
140
241
343
Z(mm)
(a) (b)
Fig. 3. Comparison between experimental results and simulated results with different fluid inlet
profiles at k
a
=1.0 (k
s
=1.0). Symbols are experimental results, and lines are simulated results.
(Solid lines correspond to the 1/7
th
power law or turbulent flow, dashed lines correspond to the
parabolic profile or laminar flow, dotted dash lines correspond to the uniform profile.)
The solid bulk viscosity
0.00 0.04 0.08 0.12 0.16
r (m)
0
1000
2000
3000
4000
5000
6000
P
(
P
a
)
292
191
89
38
Z(mm)
0.00 0.02 0.04 0.06 0.08
r (m)
-2.0
0.0
2.0
4.0
6.0
8.0
10.0
V
s
(
m
/
s
)
140
241
343
Z(mm)
(a) (b)
Fig. 4. Comparison between experimental results and simulated results with different solid bulk
viscosity at k
a
=1.0 (k
s
=1.0, 1/7
th
power law). Symbols are experimental results, and lines are
simulated results. (Solid lines correspond to zero value for the solid bulk viscosity, dashed
lines correspond to the expression from Lun et al. for the solid bulk viscosity.)
Figure 4 shows the influence of different models for estimating the solid bulk viscosity.
It is seen that, within the range of our investigations, the solid bulk viscosity almost has no
effect on simulated results. Therefore, a zero value is assigned to the solid bulk viscosity in
most of our subsequent simulations.
Restitution coefficient
The restitution coefficient is varied from 0.81 to 0.99 to study its effect on the
simulation result. Comparing with the base case with e
ss
=0.9, a 10% increase of the restitution
coefficient affects significantly on simulated results. On the other hand, a 10% decrease of the
restitution coefficient has almost no effect on the distribution of the static pressure and the
axial solid velocity. A value of 0.9, which is the typical value used in most simulations in the
literature for glass bead particles, is thus chosen and used in the simulations throughout this
work.
0.00 0.04 0.08 0.12 0.16
r (m)
0
1000
2000
3000
4000
5000
6000
P
(
P
a
)
292
191
89
38
Z(mm)
0.00 0.02 0.04 0.06 0.08
r (m)
-2.0
0.0
2.0
4.0
6.0
8.0
10.0
V
s
(
m
/
s
)
140
241
343
Z(mm)
(a) (b)
Fig. 5. Comparison between experimental results and simulated results with different
restitution coefficient at k
a
=1.0 (k
s
=1.0, 1/7
th
power law). Symbols are experimental results, and
lines are simulated results. (Solid lines correspond to e
ss
=0.9, dashed lines correspond to
e
ss
=0.81, dotted dash lines correspond to e
ss
=0.99.)
The fluid-solid exchange coefficient
0.00 0.04 0.08 0.12 0.16
r (m)
0
1000
2000
3000
4000
5000
6000
P
(
P
a
)
292
191
89
38
Z(mm)
0.00 0.02 0.04 0.06 0.08
r (m)
-2.0
0.0
2.0
4.0
6.0
8.0
10.0
V
s
(
m
/
s
)
140
241
343
Z(mm)
(a) (b)
Fig. 6. Comparison between experimental results and simulated results with different fluid-solid
exchange coefficient at k
a
=1.0 (k
s
=1.0, 1/7
th
power law). Symbols are experimental results, and
lines are simulated results. (Solid lines correspond to the fluid-solid exchange coefficient K
sl
from Gidaspow drag model, dashed lines correspond to 80% of K
sl
, dotted dash lines
correspond to 120% of K
sl
.)
Figure 6 shows the effect of the fluid-solid exchange coefficient. Within the range of
variation, there is little influence of the drag coefficient on profiles of the static pressure,
although there is a significant effect on the axial solids velocity distribution. The Gidaspow drag
model appears to be a good choice for estimating the fluid-solid exchange coefficient, and was
used throughout this study.
The axial solid phase source term
It is seen from figures 2 to 6 that the base case setting of the CFD code with proper
inlet velocity profiles, grid size, and parameters on solids bulk viscosity, restitution coefficient
and interphase exchange coefficient can properly capture the radial particle velocity
distribution profiles in the conical spouted bed. However, variations of these key parameters
failed to bring the simulation results close to the static pressure profiles. As pointed at the
beginning of the paper, the annulus region in the spouted bed cannot be treated as a fluidized
bed, and a source term needs to be introduced to correct the gravitational term in the vertical
momentum balance equation for the particle phase. The effect of the solids source term on
static pressure and axial particle velocity profiles are simulated based on equations (18) and
(19), with the simulation results shown in Fig. 7. It is seen that the axial solid phase source
term has a significant impact on the static pressure profile, but has very little effect on the
distribution of the axial solid velocity. Compared to experimental data, a selection of k
a
=0.7
seems to give the best agreement with the experimental data on the axial solid velocity, while
a slightly smaller value of k
a
gives better agreement with the static pressure data (see Fig. 8).
Therefore, a single constant value of k
a
may not be sufficient for simulating conical spouted
beds.
0.00 0.04 0.08 0.12 0.16
r (m)
0
500
1000
1500
2000
2500
3000
P
(
P
a
)
292
191
89
38
Z(mm)
0.00 0.02 0.04 0.06 0.08
r (m)
-2.0
0.0
2.0
4.0
6.0
8.0
10.0
V
s
(
m
/
s
)
140
241
343
Z(mm)
(a) (b)
Fig. 7. Comparison between experimental results and simulated results with different axial
solid phase source term (k
s
=1.0, 1/7
th
power law). Symbols are experimental results, and lines
are simulated results. (Solid lines correspond to k
a
=0.5, dashed lines correspond to k
a
=0.41,
dotted dash lines correspond to k
a
=0.7.)
0 1000 2000 3000 4000 5000
P
exp
(Pa)
0
1000
2000
3000
4000
5000
P
c
a
l
(
P
a
)
K
a
= 1
K
a
= 0.7
K
a
= 0.5
K
a
= 0.41
Fig. 8. Comparison between experimental results and simulated results with different axial
solid phase source term.
6. Conclusions
Among all factors investigated, the axial solid phase source term has the most
significant influence on static pressure profiles, followed by the restitution coefficient, with other
factors almost having no effect. Apart from the solid bulk viscosity, almost all other factors
affect the distribution of the axial solid velocity, although the effect of the axial solid phase
source term is minimal. For a complex system like the conical spouted bed, the introduction of
a source term to modify the gravitational force in the annulus region is proven to be essential,
although not perfect, in order to give reasonable agreement with the static pressure profile and
the particle velocity data.
In the spout region and fountain region, the movement of particles are quite complex,
particles were first accelerated from the bed bottom, and then decelerated in the fountain
region, thus, the drag force varies a lot in these two dilute regions because of the acceleration
and deceleration, while, these two dilute regions are simulated by fluidized beds at dynamic
balancing, and the drag force were described by Wen and Yu model (1966). Thus, to simulate
these two regions properly, more accurate models for the drag force are needed.
Notations
C
D
drag coefficient
D
0
gas inlet diameter, m
D
c
diameter of the upper cylindrical section, m
D
i
diameter of the bed bottom, m
d
s
particle diameter, m
e
ss
restitution coefficient
f drag function
g gravitational acceleration, in axial direction, the value is g=-9.81 m/s
2
; in radial
direction, the value is zero
g
0,ss
radial distribution function
H
0
static bed height, m
k
a
the ratio of the pressure drop of spouted beds to the pressure drop at stable
fluidization in the annulus region
K
ls
=K
sl
the momentum exchange coefficient between fluid phase l and solid phase s
k
s
the ratio of the pressure drop of spouted beds to the pressure drop at stable
fluidization in the spout and fountain region
n total number of phases
P static pressure, Pa
P
cal
simulation results on the static pressure, Pa
P
exp
experimental data on the static pressure, Pa
P
s
solid pressure, Pa
r radial position, m
Re
s
relative Reynolds number
Ss
solid phase source term
S
s,a
axial solid phase source term
t time, s
U
i
superficial gas velocity based on D
i
, m/s
vq
velocity of phase q, q can be fluid phase l or solid phase s, m/s
V
s
axial particle velocity, m/s
Z axial height of the bed, mm
Greek letters
q
volume fraction of phase q, q can be fluid phase l or solid phase s
l,0
loose-packed voidage
s,0
initial solid packing
s,max
packing limit
s
the granular temperature
included cone angle, degree
q
bulk viscosity of phase q, q can be fluid phase l or solid phase s, kg/(ms)
q
viscosity of phase q, q can be fluid phase l or solid phase s, kg/(ms)
s,col
solid collisional viscosity, kg/(ms)
s,fr
solid friction viscosity, kg/(ms)
s,kin
solid kinetic viscosity, kg/(ms)
l
gas density, kg/m
3
s
particle density, kg/m
3
l
fluid phase stress-strain tensor
s
solid phase stress-strain tensor
s
particulate relaxation time
Acknowledgements
This work is supported by the Natural Sciences and Engineering Research Council of
Canada (NSERC) under the Discovery Grant program.
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