21 Jinescu 3 21
21 Jinescu 3 21
21 Jinescu 3 21
https://revmaterialeplastice.ro
https://doi.org/10.37358/Mat.Plast.1964
Abstract. Some inventions along with theoretical and experimental research made it possible to increase
the output of a thermally homogeneous melt provided by the screw. However, the quality of the extruded
product depends on some specific features of the extrusion die and to a large extent on the rheological
behavior (viscous and elastic) of the polymer melt. The mismatch between the design of the screw-
cylinder subassembly and the design of the extrusion die results in products with relatively short service
life. The present paper has drawn up the working field of the extruder die and adjusted it based on the
limitations imposed by the screw-cylinder subassembly, namely: - the maximum output rate that ensures
the required thermal homogeneity of the melt; - the maximum output at which the heating system on the
barrel (and possibly the screw) ensures the extrusion temperature; - the minimum economic output
corresponding to the diameter of the screw. The working field of some extrusion dies for blown films of
the following polymers have been plotted: polypropylene, low density polyethylene, high density
polyethylene and ethylene vinyl acetate.
Keywords: extrusion of polymeric materials, extrusion die, working field of extrusion die, operating
characteristics of extrusion die and screw
Introduction
In their operation polymer processing machines thermally pollute the environment, which results,
among other things, in relatively low energy efficiency of machines operating in a polytropic mode.
On the other hand, in the case of plastics extrusion, the mismatch between the design of the screw-
cylinder subassembly and the construction of the extrusion die results in products with internal stresses
and inhomogeneous cross-section. The lifetime of these products is relatively short. In the case of pipes,
for example, fracturing before the prescribed service life can lead to the environmental pollution caused
by the substances flowing through.
Therefore, it is necessary to analyze the working field of the extrusion die considering the parameters
of the extrusion process, the behavior of the polymer melt, the conditions imposed by the quality of the
product and some economic considerations.
Extrusion machines have been improved particularly after 1953, when the first in-depth theoretical
analyses of the extrusion process were published [1-10]. The main objective was to design and
manufacture the extruder screw in such a way as to ensure the highest possible output of a thermally
homogeneous melt.
There were created spiral threaded screw barrier and then consequently intensive mixing zones on
the screw [11]. To increase the output, grooved zones were provided on the cylinder in the feed zone,
which by increasing the friction coefficient between the polymer granules and the cylinder resulted in
increased machine output [12].
Experimental and theoretical investigations in relation to the machine output, calculation relations
established for the output [13; 14], design solutions and relations corresponding to zones of intense
homogenization [15-17], as well as those related to the establishment of thermal inhomogeneity and melt
temperature variation in the screw channel [18] led to the increase of the screw potential output.
To optimize the extrusion process, initially the machine optimization diagram was plotted upon
output-pressure coordinates at the outlet of the extruder screw. Subsequently, the working field of the
extruder die was defined and plotted on the output-pressure coordinates at the extruder die inlet. The
ensuing argumentation puts forth an improved, completed version of how to define the working field of
the extruder die.
The working field adjusted to suit the limitations imposed by the screw-cylinder subassembly
becomes ABCDEFGA in Figure 2.
Next, one has to draw the characteristic of the extrusion die Gm ( pe ) at the extrusion temperature, Te,
and at temperatures Te − Te and Te + Te (Figure 3), where Te Tad represents the amplitude of the
temperature fluctuation. The allowable amplitude of temperature fluctuation Tad depends on how the
temperature influences the rheological behavior of the thermoplastic melt Materials wherein a significant
variation in viscosity occurs at a low temperature variation allow for correspondingly small values of
Tad .
Next, the functional characteristics of the screw (Gm ( pe )) are drawn, for several of its rotations
(n1; n2 nk ) , as in Figure 4. They must cross the working field of the extrusion die (Figure 5). Otherwise,
another screw, or extruder with a different diameter D shall be used (as the case may be, larger or smaller
diameters).
Possible operating points (1; 2;k ) are obtained. The operating point corresponding to the maximum
output (k ) is chosen. Intersection points outside the working field of the extrusion die (for example, 1
in Figure 5) either do not ensure the quality of the extruded product or do not provide an economically
accessible output.
The output of the extruder is proportional to the bulk density of the granular material in the inlet area
of the screw. The bulk density varies randomly between a minimum, ρ v ,min , and a maximum value,
ρ v ,max .
As a result, at a certain speed, n, the output provided by the screw, Gm, (randomly) takes values
between the curves corresponding to these two bulk densities (Figure 6). Also, because the melt
temperature randomly varies between Te − Te and Te − Te , basically three characteristics of the
extrusion die Gm,extr,die drawn, (Figure 6).
From the intersection of the two groups of extreme curves, the working micro-domain abcd and the
theoretical operating point, H, of the screw-extrusion die ensemble are obtained (Figure 6).
τ p τ cr and γ p γ cr ,
then non-uniformities appear in the product (elastic turbulence, shark skin, etc.) as a manifestation of
the elastic behavior of the viscoelastic melt [19, 20].
In the case of the non-Newtonian viscous behavior of the melt, given by the Ostwald - de Waele law,
there is a nonlinear dependence between the shear stress, τ, and the shear strain γ ,
τ = K τ γ ν , (1)
wherein K τ and are rheological constants at temperature Te, whose values for a given polymer depend
on temperature and pressure.
In the die, the pressure keeps the melt compressed. Because the melt is viscoelastic, normal stresses
σ accumulate in it. When leaving the die, in the pressure environment p0 p f , stresses σ relax, which
leads to the swelling of the product (Figure 7).
t r = lr w , (2)
+1 α +1
γ p σ
+ =1, (3)
γ
p ,cr σ cr
where γ p,cr = γ p,cr (0) is the critical wall shear rate (or velocity gradient), corresponding to p f = p0 or
σ = 0 ; σ cr - critical normal stress; υ is the exponent in law (1), while α = 1 k , where k is the exponent
featuring in the nonlinear law of melt behavior under normal stresses
σ = Kσ ε k , (4)
where K σ and k are melt constants at temperature Te, and ε – tensile strain under the action of stress σ.
It should be noted that the σ and ε of the melt are defined by natural concepts (according to Hencky) and
not by engineering concepts, being large deformations.
From relation (3) there results the critical shear rate in the case of normal stresses σ = σ( p f ) , due to
the internal melt pressure, pf,
1
σ( p f ) α +1
γ p ,cr ( p f ) = γ p ,cr (0) 1 − . (5)
σ cr
Consequently, to have a maximum value of it, it is necessary for the normal stresses to relax
completely before leaving the die.
It is useful for γ p ,cr ( p f ) to be as high as possible because the critical output through the die depends
on it.
The value of pressure pf at the die outlet decreases with an increase in the length of the die, lf (Figure
7b). For example, for a polypropylene melt at Te = 230C , it was experimentally found that
p f = 0.053 − 0.302 MPa [22].
For the die in Figure 7b the critical mass output through the die has the expression
where ρ(T ) is the melt density at the extrusion temperature and Gcr , is the volumetric critical output
d f s 2f γ p ,cr ( p f ) ,
π
Gcr = (7)
2(2 + 1 ν )
The maximum allowable output through the die (curve 5 in Figure 2) is calculated with the
relationship,
Gcr
Gad ,max = , (8)
cn
where cn 1 is a safety coefficient in relation to the critical condition at the die wall and Gcr, is the
critical output through the final zone of die (7).
By using relationship (8) one can draw the curve 5 in Figures 1 and 2.
For other curves, (3; 4) in Figure 2, one uses (Gm − pe ) dependence accounting for the whole
geometry of the flow channel through the die.
The calculated output of polypropylene blown film is from extrusion machines built in Romania.
The execution project was made at Polytechnics University of Bucharest (Project advisor V.V. Jinescu)
and implemented by Sibiu Mechanical Factory. In general, the pressure drop along the extrusion die
depends on the geometry of the channel, on the rheological behavior of the polymer melt, on the nozzle
entry effect and the elastic effects and the sliding of the melt on the wall.
The extrusion die in Figure 8, attached to an extruder with diameter D = 60 mm , has the die diameter
d f = 200 mm and a die gap thickness of s f = 0.55 and 0.65 mm. The working fields for the two different
geometries of the die, in the manufacture of polypropylene blown films are shown in Figure 8b and c. A
gap increased from 0.55mm to 0.65mm determined a shift of the curve for the maximum allowable
output to higher values, because according to relations (7) and (8) Gad ,max ~ s 2f .
On the extrusion die in Figure 9a, provided with spider mandrel, a rather narrow working field was
obtained when processing high density polyethylene (HDPE - 2) type 2 (Figure 9c).
The processing of high-density polyethylene (HDPE - 1) resulted in the working field in Figure 9, b,
with a wider working field than in Figure 9c corresponding to HPDE - 2.
When processing low density polyethylene (LDPE) on an extruder with D = 60 mm equipped with
the extrusion die in Figure 10a, one obtained the working field in Figure 10b.
Figure 10. Extrusion die for blown film attached to an extruder with D = 60 mm (a)
working field in processing low density polyethylene (LDPE) (b)
In case of the extrusion die in Figure 11a, in processing low density polyethylene (LPDE) one
obtained the relatively narrow working field in Figure 11b. In processing high density polyethylene
(HPDE -1) one obtained the operation range in Figure 11c.
When processing ethylene vinyl acetate (EVA) as a blown film on the extrusion die in Figure 12a,
the working field shown in Figure 12b, was obtained.
Figure 12. Extruder die for blown film attached to an extruder with diameter
D = 45 mm (a) working field when processing ethylene vinyl acetate (EVA) (b)
In general, to extend the working fields to higher output values, it is necessary to move vertically the
maximum allowable output curve Gad ,max This is possible, for example, by increasing γ cr ( p f ) and / or
reducing the safety coefficient cn to values close to 1.2.
From the analysis of the results obtained, represented in Figures 8 - 12, one can identify the influence
of the following parameters upon the shape and extension of the working field of the extrusion die:
- nature of processed polymeric material, individualized by the viscous and elastic behavior of its
melt
- extreme processing temperatures (Tmin ;Tmax ) ;
- type of extrusion die
- geometry of the channel through which the polymeric melt flows, especially in the final zone
(nozzle), before leaving the extrusion die
- restrictions imposed for product quality and attenuation, until disappearance, of some effects of the
elastic behavior of the polymer melt.
The operating point, the intersection of the functional characteristic of the extrusion die at the
processing temperature with the functional characteristic of the screw, depends essentially on the:
-processing temperature
-screw velocity.
Sequence of calculations for finalizing the melt path through the extrusion die
The practical solution of the problem of maximum output at an appropriate quality of the extruded
product, especially for complex cross section profiles can be done, at present, in the following stages,
which may improve, in some cases, the proposed calculation method:
– one designs of the melt path through the extrusion die (the die profile)
– one draws the operation diagram (Figure 1) of the extrusion die (zero order approximation)
– one traces the functional characteristics of the screw (Figure 4) and the functional characteristics
of the extrusion die (Figure 5)
– one establishes the effective output based on the intersection of the functional characteristics of the
screw and the extrusion die (Figure 5)
– one makes a detailed analysis (for example, by the finite element method, CAD etc.) of the
geometry of the extrusion die channels through which the melt flows (improvement in the velocity
distribution at the die exit by flow simulation as to achieve a uniform melt flow in all sections)
– one analyzes the heat transfer between the melt and the extrusion die walls and the evaluation of
the temperature profile across the thickness of the melt layer in the channel
– one corrects (adjusts) the sequence of channels in the extrusion die
– one recalculates and retraces the working field of the extrusion die (first order approximation),
the operating characteristics of the extrusion die and one determines the working point and consequently,
the output
– if the difference between the outputs of the two approximations (zero and one) is relatively large,
we move to the second order approximation and so on. In successive stages, the profile of the extrusion
die flow zones is optimized.
Conclusions
The working field of the extrusion die was delimited in the output - pressure diagram of the extrusion
die inlet (Gm - pe) by resorting to an analysis of the flow through the extrusion die, by considering the
regime parameters, the rheological behavior of the polymer melts and the influence of its elastic behavior
on the quality of the extruded product,
The working field thus obtained was adjusted by considering the flow limitations imposed by the
screw-cylinder subassembly regarding: -the minimum output corresponding to the screw diameter; - the
maximum output at which the heating system on the cylinder (and possibly inside the screw) can ensure
the intended extrusion temperature.
The interdependence between the critical shear rate and the normal internal melting stress at the die
outlet was highlighted.
Finally, there were drawn out the working fields of several extrusion dies for polyethylene (HDPE),
polypropylene (PP) and ethylene vinyl acetate (EVA) blown films.
One has detected the dependence of the extrusion die dimensions and working field extension on the
rheological behavior of the polymer and on the geometry of the path through which the viscoelastic
polymer melt flows. By applying the results obtained in this paper, the quality of the products and their
strength are improved, which has the effect of reducing the risk of premature damage.
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Manuscript received: 31.05.2021