Thermal Conductivity Behavior of Natural Fiber-Reinforced Composites

Asian Pacific Conference for Materials and Mechanics 2009 at Yokohama, Japan, November 13-16
THERMAL CONDUCTIVITY BEHAVIOR OF NATURAL

FIBER-REINFORCED COMPOSITES
Ryosuke Osugi1*, Hitoshi Takagi2, Ke Liu1, and Yusuke Gennai1

1
Graduate School of Advanced Technology and Science, The University of Tokushima
2-1 Minamijousanjima-cho, Tokushima 770-8506 Japan
2
Institute of Technology and Science, The University of Tokushima
2-1 Minamijousanjima-cho, Tokushima 770-8506 Japan
*E-mail: [email protected]
1. Introduction
Various products around us are made from plastics. One of them is fiber-reinforced plastics
(FRP). Advantages of FRP are that specific strength is bigger than that of alminium plate, and
weight of FRP is lighter than that of alminium plate, etc. Therefore, FRP are used in wide range
of fields, For example, automobile field, aerospace field, sport field, and so on. Glass-fiber
reinforced plastic (GFRP) in FRP has a lot of excellent functions such as high-strength, lightness,
and chemical stability. But, this GFRP has a serious environmental fault that disposal and
recycling are difficult after usage[1]. Recently there is study of green composites (the
biodegradable composite materials or eco-composites)[2], which are composed of a
biodegradable resin and high-strength natural fibers have been developed. There are various
Reinforced fiber. Advantages of natural fiber are low weight, they are recyclable and
biodegradable. They are also renewable and have relatively high strength and stiffness. On the
other hand, there are also some disadvantages: moisture uptake, quality variations and thermal
stability[3]. And, in fact, the mechanical property of natural fiber was much more inferior than
that of glass fiber. Therefore, essential functional strength for structural materials, or progress of
strength and toughness of green composites and securement of reliability are not enough.
Because it is necessary that the mechanical property of natural fiber approach that of glass fiber,
and natural fiber have the optional functions[4]. One of the optional functions is that natural
fibers have lumen. Lumen is hollow portion in fibers. Glass fiber and carbon fiber have used in
the past dont have lumen. These properties indicate that green composite have great thermal
insulation property. However, a lot of current studies relate to mechanical property, few studies
relate to functional property. So, we focus attention on hollow portion of natural fiber, and
examine thermal conductive property of natural fiber-reinforced composites.
2. Experomental Methods
In our study, Manila hemp fiber was used as a reinforcing fiber. This fiber has high strength
and excellent thermal stability[5]. A poly lactic acid (PLA) (Miyoshi Oil & Fat Co. Ltd., Randyi
PL-1000) and epoxy resin (Refine Tec Ltd., Epomount base resin, 9022) were used as a matrix
material. In the case of PLA, Manila hemp fiber was arrenged in one direction to preserve the
lumen. Then, the samples were prepared by mixing with PLA resin. Next, the samples were
dried for 20 hours at 70 degrees C using a circulation type oven (Toyo Seisakusho Co. Ltd.,
DRX420DA). Finally, the samples were hot pressed using a hot pressing machine (Imoto
machinery Co. Ltd., IMC-16EF). The molding was performed for 10 min at 160 degrees C and
was pressured for 10 min at 10 MPa. The samples were fabricated by altering the fiber content,
and the size of samples was 100x100x10 mm. Figure 1 shows a photograph of PLA composite
sample.
10mm
Figure 1 Photograph of PLA composites sample.
In the case of epoxy resin, Manila hemp fiber was arranged in one direction in a mold. Then,
epoxy resin was poured into the mold. The samples were unidirectional composites and the size
of sample was 100x100x10 mm. Finally, the samples were dried for 24 hours at 30 degrees C
using a circulation type oven. Thermal conductivity was measured using a steady-state method,
and perpendicular to the fiber direction. At the steady-state condition, thermal conductivity,
was calculated by the following equation:
QH QL
, (1)
TH TL 2
where is a sample thickness, Q is a heat flux, and T is a temperature. The subscripts H and L
denote high temperature part and low temperature part, respectively.
3. Results and Discussion
Figure 2 illustrates thermal conductivity of samples of PLA as a function of samples fiber
content. The thermal conductivity decreases with increasing fiber content. It is because hollow
portion of reinforced fiber contains the air. Figure 3 shows a cross-sectional view of PLA-bsed
composites sample. Thermal conductivity of the air is 0.026 [W/(mK)] at 25 degrees C. It has an
excellent heat insulation effect. The volume percent of the air increases with increasing fiber
content. Therefore, thermal conductivity decreases with increasing fiber content. The thermal
conductivity of the composites with fiber content of 76wt.% is 0.190 [W/(mK)].
4. Conclusions
Naturl fiber-reinforced composites has an excellent thermal insulation properties. The thermal
conductivity of Manila hemp fiber reinforced composites decreases with increasing fiber content.
0.4
Thermal conductivity[W/(mK)]
0.3
0.2
0.1
0
40 50 60 70 80 90 100
Weight fraction of fiber[wt.%]
Figure 2 Variation of thermal conductivity of PLA composites with weight fraction of fiber.
20m
Figure 3 Cross-sectional view of Manila hemp fiber in PLA composites.
5. References
1. Mori H., Takagi H., Hino J. and Nakaoka M., Damping Properties of Bamboo Fiber
Reinforced Eco-Composites, Journal of Ecotechnology Research, Vol. 10, No. 4, 174-175,
2004.
2. Netravali, A.N. and Chabba, S., Composites Get Greener, A Review Feature, Materials
Today, 6, 4, 22-29, 2003.
3. Oksman, K., Skrifvars, M. and Selin, J.-F., Natural fibers as reinforcement in polylactic acid
(PLA) composites, Compos Sci Technol, 63, 1317-1324, 2003.
4. Okubo, K., Takagi, H. and Goda, K., Green Composites Research and Todays Progress,
Journal of the Society of Materials Science, Japan, Vol. 55, No. 4, 438-444, 2006.
5. Ochi, S., Development of high strength biodegradable composites using Manila hemp fiber
and starch-based biodegradable resin, Composites Part A: Applied Science and
Manufacturing, Vol. 37, Issue 11, 1879-1883, 2006.

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Asian Pacific Conference for Materials and Mechanics 2009 at Yokohama, Japan, November 13-16

THERMAL CONDUCTIVITY BEHAVIOR OF NATURAL

Ryosuke Osugi1*, Hitoshi Takagi2, Ke Liu1, and Yusuke Gennai1

Figure 1 Photograph of PLA composites sample.

Figure 3 Cross-sectional view of Manila hemp fiber in PLA composites.

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